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Francis MatthewsCaptain Scarlet (voice)
Ed BishopCaptain Blue (voice)
Donald GrayCaptain White / Captain Black / The Mysterons (voice)
Cy GrantLieutenant Green (voice)
Elizabeth MorganDestiny Angel (voice)
Gary FilesCaptain Magenta / Pilot (voice)
David HealyLunar Controller / Frazer (voice)
Charles TingwellLieutenant Dean / Carter (voice)
Jeremy WilkinCaptain Ocher / Angelini / Control / Shroeder / Kurnitz / Human Captain Black (voice)
Martin KingOrson / Speech Intelligence Decoder (S.I.D.) (voice)
Sylvia AndersonLinda Nolan / Receptionist (voice)
Paul MaxwellCaptain Grey / Breck (voice)Janna Hill(voice) (credit only)Lian-Shin Yang(voice) (credit only)
