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Jack AngelPapa Smurf (voice)
Fred ArmisenBrainy (voice)
Hank AzariaGargamel (voice)
Gary BasarabaHefty (voice)
George LopezGrouchy (voice)
Melissa SturmSmurfette (voice)
Anton YelchinClumsy (voice)
Frank WelkerAzrael (voice)
Kirk BailyAdditional Voices (voice)
Jess HarnellAdditional Voices (voice)
Jeff FischerAdditional Voices (voice)
Craig KellmanAdditional Voices (voice)
John Hans TesterAdditional Voices (voice)
